Random Sequential Adsorption of Discorectangles Covered with Repulsive Shells

Authors

  • N.I. Lebovka F.D. Ovcharenko Institute of Biocolloid Chemistry, Nat. Acad. of Sci. of Ukraine
  • L.A. Bulavin Taras Shevchenko National University of Kyiv, Faculty of Physics
  • M.R. Petryk Ivan Pulyui National Technical University of Ternopil
  • N.V. Vygornitskii F.D. Ovcharenko Institute of Biocolloid Chemistry, Nat. Acad. of Sci. of Ukraine

DOI:

https://doi.org/10.15407/ujpe69.5.357

Keywords:

adsorption, two-dimensional films, jamming, interparticle interactions

Abstract

Adsorption of anisometric particles (discorectangles) on a two-dimensional substrate has been studied. The aspect ratio (the length-to-width ratio ɛ = l/d) was changed within the interval ɛ = 1–10. A modified random sequential adsorption (RSA) model is studied. In this model, the particles were covered with repulsive shells. The main parameters of the model are the thickness Rc of the permeable shell and the maximum number Zm of the shells of the nearest particles that can be crossed by the shell of the next deposited particle. The behavior of the degree of surface coverage in the saturated (jammed) state at various values of the parameters Rc, Zm, and ɛ is discussed.

References

N.I. Lebovka, Y.Y. Tarasevich. Two-dimensional systems of elongated particles: From diluted to dense. In: Order, Disorder and Criticality. Edited by Y. Holovatch (World Scientific, 2020), vol. 6, p. 30.

https://doi.org/10.1142/9789811216220_0004

P. Krapivsky. Random sequential covering. J. Stat. Mech. Theor.Exper. 2023, 033202 (2023).

https://doi.org/10.1088/1742-5468/acbc20

A. Renyi. On a one-dimensional problem concerning random space-filling problem. Publ. Math. Inst. Hungar. Acad.Sci. 3, 109 (1958).

J. Feder. Random sequential adsorption. J. Theor. Biol. 87, 237 (1980).

https://doi.org/10.1016/0022-5193(80)90358-6

P. Kubala, P. Batys, J. Barbasz, P. Weronski, M. Cie'sla. Random sequential adsorption: An efficient tool for investigating the deposition of macromolecules and colloidal particles. Adv. Colloid Interf. Sci. 306, 102692 (2022).

https://doi.org/10.1016/j.cis.2022.102692

K. Haiduk, P. Kubala, M. Ciesla. Saturated packings of convex anisotropic objects under random sequential adsorption protocol. Phys. Rev. E 98, 63309 (2018).

https://doi.org/10.1103/PhysRevE.98.063309

N.I. Lebovka, N.V. Vygornitskii, Y.Yu. Tarasevich. Random sequential adsorption of partially ordered discorectangles onto a continuous plane. Phys. Rev. E 102, 022133 (2020).

https://doi.org/10.1103/PhysRevE.102.022133

J.W. Evans. Random and cooperative sequential adsorption. Rev. Mod. Phys. 65, 1281 (1993).

https://doi.org/10.1103/RevModPhys.65.1281

A. Cadilhe, N.A.M. Ara'ujo, V. Privman. Random sequential adsorption: from continuum to lattice and prepatterned substrates. J. Phys.: Condens. Matter 19, 065124 (2007).

https://doi.org/10.1088/0953-8984/19/6/065124

Z. Adamczyk. Particle adsorption and deposition: role of electrostatic interactions. Adv. Colloid Interf. Sci. 100, 267 (2003).

https://doi.org/10.1016/S0001-8686(02)00062-3

Z. Adamczyk, P. Weronski, E. Musial. Colloid particle adsorption on partially covered (random) surfaces. J. Colloid Interf. Sci. 241, 63 (2001).

https://doi.org/10.1006/jcis.2001.7601

M. Sadowska, M. Cie'sla, Z. Adamczyk. Nanoparticle deposition on heterogeneous surfaces: Random sequential adsorption modeling and experiments. Colloid. Surface. A 617, 126296 (2021).

https://doi.org/10.1016/j.colsurfa.2021.126296

N.I. Lebovka, M.O. Tatochenko, N.V. Vygornitskii, Y.Yu. Tarasevich, Confinement effects on the random sequential adsorption packings of elongated particles in a slit, Phys. Rev. E 104, 054104 (2021).

https://doi.org/10.1103/PhysRevE.104.054104

N.I. Lebovka, M.R. Petryk, M.O. Tatochenko, N.V. Vygornitskii. Two-stage random sequential adsorption of discorectangles and disks on a two-dimensional surface. Phys. Rev. E 108, 024109 (2023).

https://doi.org/10.1103/PhysRevE.108.024109

Published

2024-06-26

How to Cite

Lebovka, N., Bulavin, L., Petryk, M., & Vygornitskii, N. (2024). Random Sequential Adsorption of Discorectangles Covered with Repulsive Shells. Ukrainian Journal of Physics, 69(5), 357. https://doi.org/10.15407/ujpe69.5.357

Issue

Section

Surface physics

Most read articles by the same author(s)

<< < 1 2 3 4 5 > >>