Determination of the 93Zr and 93Mo Isotope Contents in NPP-Produced Radioactive Materials

Authors

  • V.O. Zheltonozhsky Institute for Nuclear Research, Nat. Acad. of Sci. of Ukraine
  • D.E. Myznikov Institute for Nuclear Research, Nat. Acad. of Sci. of Ukraine
  • A.M. Savrasov Institute for Nuclear Research, Nat. Acad. of Sci. of Ukraine
  • V.I. Slisenko Institute for Nuclear Research, Nat. Acad. of Sci. of Ukraine
  • L.V. Sadovnikov Institute for Nuclear Research, Nat. Acad. of Sci. of Ukraine

DOI:

https://doi.org/10.15407/ujpe69.9.625

Keywords:

flux-weighted average yields, photoactivation method, gamma spectrometry, zirconium, molybdenum, cobalt

Abstract

A photoactivation method for determining the produced activities of 93Zr and 93Mo isotopes has been developed. The method consists of irradiating the metals and sorbents of radioactive materials produced at the Zaporizhzhya NPP with bremsstrahlung γ-quanta with an end-point energy of 18.5 MeV. From the measured γ-spectra and using the yield ratios for 99Mo, 58Co, and 89Zr isotopes, the 92Mo/59Co and 92Zr/59Co concentration ratios were determined. From the obtained data and the measured produced activity of 60Co isotopes in the studied specimens, the overall activities of 93Zr and 93Mo isotopes are calculated.

References

J.C. Evans et al. Long-Lived Activation Products in Reactor Materials (Pacific Northwest Laboratory, 1984).

https://doi.org/10.2172/6776358

V.A. Zheltonozhsky, D.E. Myznikov, V.I. Slisenko, M.V. Zheltonozhskaya, A.P. Chernyaev. Determination of the long-lived 10Be in construction materials of nuclear power plants using photoactivation method. J. Environ. Radioactiv. 227, 106509 (2021).

https://doi.org/10.1016/j.jenvrad.2020.106509

R.B. Firestone. Table of Isotopes. 8th Edition (Wiley Interscience, 1996).

A.I Abramov, Yu. A. Kazanskii, E.S. Matusevich. Fundamentals of Experimental Methods of Nuclear Physics (Energoatomizdat, 1985) (in Russian).

E.A. Zhyrbenko, B.K. Bulkin. The main approaches to determining the activity of the structures of reactor units with VVER during their decommissioning. In: Proceedings of the 6th International Scientific and Technical Conference "Safety Assurance of NPP with VVER", Podolsk, May 26-29, 2009 (OKB Gidropress, 2009), p. 1 (in Russian).

S.P. Kapica, V.N. Melekhin. The Microtron (Harwood Academic, 1978).

J.F. Briesmeister. MCNP-A General Monte Carlo N-Particle Transport Code. Report LA-12625-M (Los Alamos National Laboratory, 1997).

S. Agostinelli et al. GEANT4 - a simulation toolkit. Nucl. fInstrum. Methods. A 506, 250 (2003).

A.J. Koning, D. Rochman. Modern nuclear data evaluation with the TALYS code system. Nucl. Data Sheets 113, 2841 (2012).

https://doi.org/10.1016/j.nds.2012.11.002

V.O. Zheltonozhsky, D.E. Myznikov, A.M. Savrasov, V.I. Slisenko, Determination of the activity of 63Ni in NPP structural materials. Nucl. Phys. At. Energ. 23, 207 (2022) (in Ukrainian).

https://doi.org/10.15407/jnpae2022.03.207

H. Beil, R. Bergere, P. Carlos, A. Lepretre, A. de Miniac, A. Veyssiere. A study of the photoneutron contribution to the giant dipole resonance in doubly even Mo isotopes, Nucl. Phys. A 227, 427 (1974).

https://doi.org/10.1016/0375-9474(74)90769-6

B.L. Berman, J.T. Caldwell, R.R. Harvey, M.A. Kelly, R.L. Bramblett, S.C. Fultz. Photoneutron cross sections for 90Zr, 91Zr, 92Zr, 94Zr, and 89Y. Phys. Rev. 162, 1098 (1967).

S.C. Fultz, R.L. Bramblett, J.T. Caldwell, N.E. Hansen, C.P. Jupite. Photoneutron cross-sections for 51V and 59Co. Phys. Rev. 128, 2345 (1962).

J. Kopecky. Atlas of Neutron Capture Cross Sections (JUKO Research, 1997).

V.O. Zheltonozhsky, D.E. Myznikov, A.M. Savrasov, V.I. Slisenko Determination of 59Ni and 55Fe contents in NPP structural elements. Ukr. J. Phys. 67, 707 (2022).

https://doi.org/10.15407/ujpe67.10.707

Published

2024-10-16

How to Cite

Zheltonozhsky, V., Myznikov, D., Savrasov, A., Slisenko, V., & Sadovnikov, L. (2024). Determination of the 93Zr and 93Mo Isotope Contents in NPP-Produced Radioactive Materials. Ukrainian Journal of Physics, 69(9), 625. https://doi.org/10.15407/ujpe69.9.625

Issue

Section

Fields and elementary particles

Most read articles by the same author(s)